Polyaromatic Hydrocarbons

A) US EPA List of Priority pollutants contains 16 polyaromatic hydrocarbons. Reliable sublimation pressures and enthalpies for 9 compounds from this list were already published in our laboratory:
naphthalene [1], acenaphthylene , fluorene, fluoranthene [2], acenaphthene, pyrene, phenanthrene, benzo[a]pyrene [3], anthracene [4].
Sublimation pressures for remaining 7 compounds are planned to be determined in near future: chrysene, benzo[a]anthracene, benzo[b]fluoranthene, benzo[k]fluoranthene, dibenzo[a,h]anthracene, indeno[1,2,3-c,d]pyrene, benzo[g,h,i]perylene. We already measured heat capacities for several compounds from this list [5]

B) Also other PAHs and PAH-related distillation cuts were studied [6-10].

References

[1] Růžička, K.; Fulem, M.; Růžička, V., Recommended Vapor Pressure of Solid Naphthalene. Journal of Chemical and Engineering Data 2005, 50, (6), 1956-1970  https://doi.org/10.1021/je050216m

[2]. Mahnel, T., V. Štejfa, M. Fulem, K. Růžička, Recommended vapor pressures for acenaphthylene, fluoranthene, and fluorene. Fluid Phase Equilibria, 2017. 434: p. 74-86.  https://doi.org/10.1016/j.fluid.2016.11.012

[3] Růžička, K.; Mokbel, I.; Majer, V.; Růžička, V.; Jose, J.; Zábranský, M., Description of vapor-liquid and vapor-solid equilibria for a group of polycondensed compounds of petroleum interest. Fluid Phase Equilibria 1998, 148, (1-2), 107-137.  https://doi.org/10.1016/S0378-3812(98)00200-3
(acenaphthene, pyrene, phenanthrene, benzo[a]pyrene, vapor pressures measured in Lyon)

[4]  Mahnel T.; Štejfa V.; Maryška M.; Fulem M.; Růžička K.,
Reconciled thermophysical data for anthracene. Journal of Chemical Thermodynamics, 2019, 129, 61-72.  https://doi.org/10.1016/j.jct.2018.08.034

[5] Mahnel T.; Pokorný V.; Fulem M.; Sedmidubský D.; Růžička K.,
Measurement of low-temperature heat capacity by relaxation technique: Calorimeter performance testing and heat capacity of benzo[b]fluoranthene, benzo[k]fluoranthene, and indeno[1,2,3-cd]pyrene. The Journal of Chemical Thermodynamics, Volume 142, January 2020, 105964 https://doi.org/10.1016/j.jct.2019.105964

[6] Fulem, M.; Laštovka, V.; Straka, M.; Růžička, K.; Shaw, J. M., Heat Capacities of Tetracene and Pentacene. Journal of Chemical and Engineering Data 2008, 53, (9), 2175-2181 https://doi.org/10.1021/je800382b

[7] Bazyleva, A., M. Fulem, M. Becerra, B. Zhao, J.M. Shaw, Phase Behavior of Athabasca Bitumen. Journal of Chemical and Engineering Data, 2011. 56(7): p. 3242-3253. https://doi.org/10.1021/je200355f

[8] Sánchez-Lemus, M.C., F. Schoeggl, S.D. Taylor, K. Růžička, M. Fulem, H.W. Yarranton, Deep-Vacuum Fractionation of Heavy Oil and Bitumen, Part II: Interconversion Method. Energy & Fuels, 2014. 28(5): p. 2866-2873. https://doi.org/10.1021/ef500490h 

[9] Sanchez-Lemus, M.C., F. Schoeggl, S.D. Taylor, T. Mahnel, P. Vrbka, K. Růžička, M. Fulem, H.W. Yarranton, Vapor pressure and thermal properties of heavy oil distillation cuts. Fuel, 2016. 181: p. 503-521. https://doi.org/10.1016/j.fuel.2016.04.143

[10] Štejfa V., Mahnel T., Skořepová E., Rohlíček J., Eigner V., Schröder B., Růžička K., Fulem M.
A combined thermodynamic and crystallographic study of 1,3-diisopropylnaphthalene.
The Journal of Chemical Thermodynamics, 150, 2020, 106193, https://doi.org/10.1016/j.jct.2020.106193


Laboratory of Applied Thermodynamics | UCT Prague
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